magnetic materials have attracted significant attention owing to their highly tunable physical properties and potential applications in novel spintronics. Some of them can still exhibit intrinsic long-range magnetic order when they are exfoliated even into a few layers, such as ferromagnetic semiconductor CrSiTe₃ with a centrosymmetric layered structure.

Both superconductivity and enhancement of ferromagnetism, usually competing for orders, have been observed in CrSiTe₃ at high pressure. However, the high-pressure structure of CrSiTe₃ is still unclear, setting obstacles in understanding pressure-induced novel physics.

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